Considering the length of the cable run, that's probably a good choice if you want 100 amps. Many folks use dual rated 2-2-2-4 AL MHF because its less expensive and easy to find in stock, although its only rated for 90 amps.
I ran 2" for the electrical conduit and IIRC I used 1.5" for the low voltage conduit. It took a fair amount of lubricant and pulling to get 2-2-2-4 MHF through 2" 90 degree long sweep bends, but it was simple through the straight section. My wire was dual rated for inside use and burial (I think the wire in your link is also), so I could run it in conduit right into my subpanel.
The four MHF wires came bundled, with a piece of fiberglass tape every few feet to keep them together. Keep track of the junctions in your conduit, and pull the wire in a direction that does not catch on the lip where the conduit is glued together. That lip looks really small, but does a good job of catching the tape around the individual wires. Make sure you include a new pull string in both conduits, so you can go back later if needed.
Bruce