OK, I've looked at the replies in some detail and I'm going to attempt to reply to wyliesdiesels' comments particularly and see if I can articulate correctly a plan of action. I've placed wyliesdiesels' comments below in red with my follow up commentary/questions below.
In regards to the Main Service Panel feed to the Old Shop Sub Panel:
To clarify, if you look closely at the schematic, you'll notice the two Neutral bus bars are bonded together, but isolated from the ground bus bar which is actually bonded to the panel. So, the neutral is NOT bonded to the can. Hence, I'm thinking to this point, this is all correct and to code (current and past).
In regards to the Old Shop Sub Panel feed to the Apartment Sub Panel:
To clarify, there are NO metallic pathways to the Apartment structure. In fact, all sub panels in the separate structures have no metallic pathways between them. I understand that it was to code PRE-2008 as a three wire feed and I further understand that the grounding electrodes are for shunting lightning.
Question: To be clear, using PRE-2008 code criteria, the Apartment Sub Panel which has a 3-wire feed is OK to the old criteria (considering no metallic pathways exist between structures) as long as I install a grounding electrode for shunting lightning?
In regards to the Old Apartment Sub Panel feed to the Pump House:
I acknowledge, understand, and appreciate the comments about the bare copper wire being incorrectly used as a neutral. I also understand the following comments about the dangers of not rectifying this condition. Frankly, my discovery of the bare copper wire being used as a neutral was the root cause of my beginning this thread in the first place.
And I feel the only really good solution is to run a new 4 wire feed to the pump house from the Apartment. This way, I could re-wire a proper sub panel in the pump house using dedicated, separate, ground and neutral conductors.
So, in summary, given the clarification above about the Old Shop sub panel (i.e. the neutral bus is not bonded to the ground and can there), I'm considering the following actions:
1) Adding a grounding electrode at the Apartment for shunting lightning and bringing that sub panel to PRE-2008 code compliance; and,
2) Replacing the feed from the Apartment to the Pump House with new 4-wire feed which would then allow me to re-wire the sub panel in the pump house considering the separated ground and neutral at that location. I'll also take this opportunity to properly install the 120V outlet with a lower circuit breaker inline.
Does the above statement of planned actions make sense and seem prudent given my conditions?
Your insight and help is, as always, most appreciated.
Regards, Jimt1000